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Hybrid Magnonics in Hybrid Perovskite Antiferromagnets

April 1, 2023

Layered hybrid perovskite antiferromagnets with an interlayer Dzyaloshinskii—Moriya-Interaction (DMI) can lead to a strong intrinsic magnon-magnon coupling strength up to 0.24 GHz, which is four times greater than the dissipation rates of the acoustic/optical modes. This work shows that the DMI in these hybrid antiferromagnets holds promise for leveraging magnon-magnon coupling by harnessing symmetry breaking in a highly tunable, solution-processable layered magnetic platform.

Scientific Achievement

Hybrid magnonic systems are a newcomer for pursuing coherent information processing owing to their rich quantum engineering functionalities. Generally, hybrid magnonics are forbidden due to their opposite parity. Here we show that the DMI, a chiral antisymmetric interaction that occurs in magnetic systems with low symmetry, can lift this restriction. We report that layered hybrid perovskite antiferromagnets (HOIP-AFMs) with an interlayer DMI can lead to a strong intrinsic magnon-magnon coupling.

Significance and Impact

Our work shows that the DMI in these HOIP-AFMs holds promise for leveraging hybrid magnonics by harnessing symmetry breaking in a highly tunable, solution processable layered magnetic platform.

Research Details

  • A large, intrinsic, exceptional magnon-magnon coupling in a new HOIP-AFMs platform has a more accessible frequency range (i.e., GHz).
  • An optical magnon mode (dark magnon) existing far above the saturation field is observed, activated by antisymmetric nature of the DMI.

DOI:  https://doi.org/10.1038/s41467-023-37505-w

Related People

Matthew Beard
National Renewable Energy Laboratory

Dali Sun
North Carolina State University

A diagram showing broken symmetry and a chart showing the frequency (GHz) of magnetic field.